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Spectroscopic Investigations of Hydrogen Bond Network Structures in Water Clusters, 2013 Springer Theses Series

Langue : Anglais

Auteur :

Couverture de l’ouvrage Spectroscopic Investigations of Hydrogen Bond Network Structures in Water Clusters
The properties and nature of water clusters studied with novel spectroscopic approaches are presented in this thesis. Following a general introduction on the chemistry of water and water clusters, detailed descriptions of the experiments and analyses are given. All the experimental results, including first size-selective spectra of large clusters consisting of 200 water molecules, are presented with corresponding analyses. Hitherto unidentified hydrogen bond network structures, dynamics, and reactivity of various water clusters have been characterized at the molecular level. The main targets of this book are physical chemists and chemical physicists who are interested in water chemistry or cluster chemistry.

General Introduction.- Infrared spectroscopy of chromophore-labeled water clusters phenol-(H2O)n (n < ~50).- Infrared pectroscopy of large protonated water clusters H+(H2O)n (n ≤ 221).- Tuning of the Internal Energy and Isomer Distribution in Protonated Water Clusters H+(H2O)n (n ≤ 50): Towards a more detailed understanding of structures and dynamics.- Infrared spectroscopy of water cluster radical cations (H2O)n+ (n ≤ 11).- Conclusions and future work.

Kenta Mizuse, Ph.D.

Date of Birth: February 16, 1984

Place of Birth: Niigata, Japan

Nationality: Japan

 

Since April 2011

Department of Photo-Molecular Science (Prof. Yasuhiro Ohshima’s Lab.), Institute for Molecular Science, Japan

Assistant professor

 

April 2008-March 2011

The Japan Society for the Promotion of Science (JSPS) Research fellow

 

April 2006-March 2011

Department of Chemistry, Graduate School of Science, Tohoku University, Japan

Ph.D. student

Supervisor: Professor Asuka Fujii

Degree obtained: Ph.D. in Science

 

April 2002-March 2006

Department of Chemistry, Faculty of Science, Tohoku University, Japan

Undergraduate student

Supervisor: Professor Naohiko Mikami

 

Publications

1                Mizuse, K. & Fujii, A. Infrared Spectroscopy of Large Protonated Water Clusters H+(H2O)20-50 Cooled by Inert Gas Attachment. Chem. Phys.in press, doi:10.1016/j.chemphys.2012.07.012 (2013).

2                Mizuse, K. & Fujii, A. Tuning of the Internal Energy and Isomer Distribution in Small Protonated Water Clusters H+(H2O)4–8: An Application of the Inert Gas Messenger Technique. J. Phys. Chem. A116, 4868-4877 (2012).

3                Mizuse, K., Suzuki, Y., Mikami, N. & Fujii, A. Solvation-Induced σ-Complex Structure Formation in the Gas Phase: A Revisit to the Infrared Spectroscopy of [C6H6–(CH3OH)2]+. J. Phys. Chem. A115, 11156-11161 (2011).

4                Mizuse, K., Kuo, J.-L. & Fujii, A. Structural trends of ionized water networks: Infrared spectroscopy of water cluster radical cations(H2O)n+ (n = 3-11). Chem. Sci.2, 86

Nominated by Tohoku University as an outstanding Ph.D. thesis Novel experimental methods for structural analyses of very large water clusters are presented New chemical models for radiation-induced reactions in water are reported Includes supplementary material: sn.pub/extras

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Date de parution :

Ouvrage de 175 p.

15.5x23.5 cm

Disponible chez l'éditeur (délai d'approvisionnement : 15 jours).

Prix indicatif 105,49 €

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